CHAPTER 8: Question 9
Simple Answers
The slow step (and hence the rate determining step) of this reaction
involves attack of hydroxide on the carbonyl bond. Hence, in the transition
state of this step of the reaction, the acetate group is converted into
a larger substituent since it is interacting with the hydroxide. In the
trans-isomer (A), the acetate is in an equatorial
position, whilst in the cis-isomer (A) the acetate group has to adopt
an axial position. Substituents in axial positions are less stable than
those in equatorial positions for steric reasons, and this destabilisation
increases as the size of the group increases. Hence, although isomer B
is less stable than isomer A, the energy difference between the starting
material and transition state for B is greater than the corresponding energy
difference for isomer A. Since it is the energy difference between the
starting material and transition state (the activation energy) that determines
the rate of reaction, A is hydrolysed more rapidly than B. This is illustrated
graphically
below.
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